Jul 7 – 11, 2025
Europe/Bratislava timezone
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Investigating Quantum States in Spin Chain Materials

I-03
Jul 7, 2025, 3:00 PM
30m
INVITED ORAL Topic 4 - Magnetic materials and heterostructures for spintronics, topological and quantum magnetic phenomena Invited talks

Speaker

Bella Lake (Helmholtz Zentrum Berlin, Germany)

Description

The antiferromagnetic spin-$1/2$ spin chain with Heisenberg-Ising (XXZ) anisotropy is a rich source of novel phenomena. Good physical realizations are the compounds SrCo$_2$V$_2$O$_8$ and BaCo$_2$V$_2$O$_8$ where the Co$^{2+}$ ions have effective spin-$1/2$ and are coupled by antiferromagnetic interactions into chains while collinear long-range magnetic order occurs below $T_N\approx 5$ K due to weak interchain coupling. In a longitudinal magnetic field applied along the easy axis, the magnetic order is suppressed and using inelastic neutron scattering and optical spectroscopy we find the evidence for complex bound states of magnetic excitations, known as Bethe strings. Furthermore, the characteristic energy, scattering intensity and linewidth of the observed string states exhibit excellent agreement with precise Bethe ansatz calculations. Our results confirm the existence of the long-sought Bethe string excitations predicted almost a century ago. Application of transverse magnetic field along the direction perpendicular to the easy axis induces a quantum phase transition where the antiferromagnetic order is destroyed at a three-dimensional quantum critical point. The evolution of the excitations is investigated as a function of field revealing a complex series of modes and continuum scattering which are compared to theory. At a particular field still within the antiferromagnetically ordered phase we find a sequence of excitations whose energies match the predictions based on the E$8$ Lie group symmetry.

Acknowledgements

Funding was provided by Helmholtz Gemeinschaft.

Primary author

Konrad Puzniak (Helmholtz-Zentrum Berlin fur Materialien und Energie, Berlin, Germany.)

Co-authors

A.K. Bera (Helmholtz-Zentrum Berlin fur Materialien und Energie, Berlin, Germany.) Nazmul Islam (Helmholtz-Zentrum Berlin fur Materialien und Energie, Berlin, Germany.) J. Ma (Tsung-Dao Lee Institute, Shanghai Jiao Tong University, Shanghai, China.) J. Wu (Tsung-Dao Lee Institute, Shanghai Jiao Tong University, Shanghai, China.) W. Yang (Stewart Blusson Quantum Matter Institute, Vancouvepr, British Columbia, Canada.) Z. Wang (Institute of Physics II, University of Cologne, Cologne, Germany.) X. Wang (Tsung-Dao Lee Institute, Shanghai Jiao Tong University, Shanghai, China.) M. Bartkowiak (Helmholtz-Zentrum Berlin fur Materialien und Energie, Berlin, Germany.) O. Prokhnenko (Helmholtz-Zentrum Berlin fur Materialien und Energie, Berlin, Germany.) B. Klemke (Helmholtz-Zentrum Berlin fur Materialien und Energie, Berlin, Germany.) R. Bewley (ISIS Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, UK.) C. Balz (ISIS Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, UK.) M. Boehm (Institut Laue–Langevin, Grenoble, France) J. Xu (Helmholtz-Zentrum Berlin fur Materialien und Energie, Berlin, Germany.) K. Schmalzl (Jülich Centre for Neutron Science, at ILL, Grenoble, France) M. Matsuda (Neutron Scattering Division, Oak Ridge National Laboratory, Tennessee 37831, USA) A. Okutani (Center for Advanced High Magnetic Field Science, Osaka University, Osaka 560-0043, Japan) M. Hagiwara (Center for Advanced High Magnetic Field Science, Osaka University, Osaka 560-0043, Japan) Bella Lake (Helmholtz Zentrum Berlin, Germany)

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