21–23 May 2025
Belgrade
Europe/Belgrade timezone

Electric field control of spin (and valley) polarization in two-dimensional antiferromagnets

22 May 2025, 14:15
30m
Science Technology Park (Belgrade)

Science Technology Park

Belgrade

Veljka Dugosevica 54, 11050 Belgrade, Serbia
Invited Oral 3. Antiferromagnetic and altermagnetic 2D materials thursday afternoon

Speaker

Marco Gibertini

Description

Antiferromagnetic conductors with suitably broken spatial symmetries host spin-polarized bands even in the absence of spin-orbit coupling, leading to transport phenomena commonly observed in metallic ferromagnets. Here we show that, in the two-dimensional (2D) limit, an electric field can control the relevant symmetries. Two situations are discussed. First, we show by first-principles simulations and magnetotransport experiments that a perpendicular electric displacement field can switch the spin polarization of the conduction band on and off in an antiferromagnetic van der Waals bilayer, such as CrPS$_4$. Second, we consider the case of altermagnets, where spin-valley locking can give rise to band extrema (valleys) at different locations in the Brillouin zone for opposite spins. By screening high-throughput databases of 2D magnetic materials, we find a potential candidate with suitable symmetries, where an electric field can lift the degeneracy between valleys with opposite spin and thus create a simultaneous spin and valley polarization. First-principles simulations predict a sizeable effect that meets the requirements for applications in spin-valleytronics.

Acknowledgements

We acknowledge financial support from Ministero Italiano dell'Università e della Ricerca through the PRIN2022 project SECSY (CUP E53D23001700006), funded by the European Union – NextGenerationEU.

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